Unable to Boot/Login after Crash during upgrade

Well, the error you quoted makes two points obvious:

1. The current theme cannot be loaded
2. module "org.kde.kirigami" is not installed

You could try installing kirigami (from within a chroot environment) to see if that might resolve the issue.

sudo pacman -S kirigami

As is said, “nothing ventured, nothing gained”; however, the hard reset you described might have damaged anything; it’s difficult to predict.

Usually, in similar situations we might suggest working through a tutorial such as Recovering from an Interrupted Update/Upgrade, the general gist of which seems not unlike what you have already tried, yourself.

Mentioned earlier was to run the update again from chroot; this can’t hurt. As you seem to be more inclined to use pamac-cli, you could try the following:

pamac update --no-aur --force-refresh

and if that succeeds;

pamac update --aur

(if you have installed software from the AUR) and;

flatpak update

(again, optional)

Reboot and see what the status is then.